Field-Emission Resonances in Thin Metallic Films: Nonexponential Decay of the Tunneling Current as a Function of the Sample-to-Tip Distance
| Autor: | Aladyshkin, A. Yu., Schouteden, K. |
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| Rok vydání: | 2023 |
| Předmět: | |
| Zdroj: | Journal of Physical Chemistry C, vol. 126, 13341-13348 (2022) |
| Druh dokumentu: | Working Paper |
| DOI: | 10.1021/acs.jpcc.2c02374 |
| Popis: | Field-emission resonances (FERs) for two-dimensional Pb(111) islands grown on \mbox{Si(111)7$\times$7} surfaces were studied by low-temperature scanning tunneling microscopy and spectroscopy (STM/STS) in a broad range of tunneling conditions with both active and disabled feedback loop. These FERs exist at quantized sample-to-tip distances $Z^{\,}_n$ above the sample surface, where $n$ is the serial number of the FER state. By recording the trajectory of the STM tip during ramping of the bias voltage $U$ (while keeping the tunneling current $I$ fixed), we obtain the set of the $Z^{\,}_n$ values corresponding to local maxima in the derived $dZ/dU(U)$ spectra. This way, the continuous evolution of $Z^{\,}_n$ as a function of $U$ for all FERs was investigated by STS experiments with active feedback loop for different $I$. Complementing these measurements by current-distance spectroscopy at a fixed $U$, we could construct a 4-dimensional $I-U-Z-dZ/dU$ diagram, that allows us to investigate the geometric localization of the FERs above the surface. We demonstrate that (i) the difference $\delta Z^{\,}_n=Z^{\,}_{n+1}-Z^{\,}_n$ between neighboring FER lines in the $Z-U$ diagram is independent of $n$ for higher resonances, (ii) the $\delta Z^{\,}_{n}$ value decreases as $U$ increases; (iii) the quantized FER states lead to the \emph{periodic} variations of $\ln I$ as a function of $Z$ with periodicity $\delta Z$; (iv) the periodic variations in the $\ln I - Z$ spectra allows to estimate the absolute height of the tip above the sample surface. Our findings contribute to a deeper understanding on how the FER states affect various types of tunneling spectroscopy experiments and how they lead to a non-exponential decay of the tunneling current as a function of $Z$ at high bias voltages in the regime of quantized electron emission. Comment: 25 pages, 18 figures |
| Databáze: | arXiv |
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