Pressure-induced nontrivial $Z_2$ band topology and superconductivity in transition metal chalcogenide $\mathrm{Ta}_2 \mathrm{Ni}_3 \mathrm{Te}_5$

Autor: Yang, Haiyang, Zhou, Yonghui, Wang, Shuyang, Wang, Jing, Chen, Xuliang, Zhang, Lili, Xu, Chenchao, Yang, Zhaorong
Rok vydání: 2023
Předmět:
Zdroj: Physical Review B 107, L020503 (2023)
Druh dokumentu: Working Paper
DOI: 10.1103/PhysRevB.107.L020503
Popis: The unique electronic and crystal structures driven by external pressure in transition metal chalcogenides (TMCs) can host emergent quantum states. Here we report pressure-induced metallization, nontrivial $Z_2$ band topology and superconductivity in TMC $\mathrm{Ta}_2 \mathrm{Ni}_3 \mathrm{Te}_5$. Our electrical transport measurements show that the metallization emerges at 3.3 GPa, followed by appearance of the superconductivity at $P_{\mathrm{c}}$ = 21.3 GPa with $T_{\mathrm{c}} \sim$ 0.4 K. Room-temperature synchrotron x-ray diffraction experiments demonstrate the stability of the pristine orthorhombic structure upon compression. Our first-principles calculations further reveal a topological phase transition (from $Z_2=0$ to $Z_2=1$), which occurs after $\mathrm{Ta}_2 \mathrm{Ni}_3 \mathrm{Te}_5$ is turned into an electron-hole compensated semimetal by pressure. The pressure-induced superconductivity at $P_{\mathrm{c}}$ could be attributed to the abruptly enhanced density of states at the Fermi level. These findings demonstrate that $\mathrm{Ta}_2 \mathrm{Ni}_3 \mathrm{Te}_5$ is a new platform for realizing exotic quantum phenomena in TMCs, as well as exploring the interplay between topological property and superconductivity.
Comment: 6 pages, 6 figures. arXiv admin note: text overlap with arXiv:2301.09050
Databáze: arXiv