Electronic band structure in pristine and Sulfur-doped Ta$_2$NiSe$_5$

Autor: Saha, Tanusree, Petaccia, Luca, Ressel, Barbara, Ribič, Primož Rebernik, Di Santo, Giovanni, Zhao, Wenjuan, De Ninno, Giovanni
Rok vydání: 2022
Předmět:
Druh dokumentu: Working Paper
DOI: 10.1103/PhysRevB.106.075148
Popis: We present an angle-resolved photoemission study of the electronic band structure of the excitonic insulator Ta$_2$NiSe$_5$, as well as its evolution upon Sulfur doping. Our experimental data show that while the excitonic insulating phase is still preserved at a Sulfur-doping level of 25$\%$, such phase is heavily suppressed when there is a substantial amount, $\sim$ 50$\%$, of S-doping at liquid nitrogen temperatures. Moreover, our photon energy-dependent measurements reveal a clear three dimensionality of the electronic structure, both in Ta$_2$NiSe$_5$ and Ta$_2$Ni(Se$_{1-x}$S$_x$)$_5$ ($x=0.25, 0.50$) compounds. This suggests a reduction of electrical and thermal conductivities, which might make these compounds less suitable for electronic transport applications.
Databáze: arXiv