Extreme ultraviolet wave packet interferometry of the autoionizing HeNe dimer

Autor:	Uhl, Daniel, Wituschek, Andreas, Michiels, Rupert, Trinter, Florian, Jahnke, Till, Allaria, Enrico, Callegari, Carlo, Danailov, Miltcho, Di Fraia, Michele, Plekan, Oksana, Bangert, Ulrich, Dulitz, Katrin, Landmesser, Friedemann, Michelbach, Moritz, Simoncig, Alberto, Manfredda, Michele, Spampinati, Simone, Penco, Giuseppe, Squibb, Richard James, Feifel, Raimund, Laarmann, Tim, Mudrich, Marcel, Prince, Kevin C., Cerullo, Giulio, Giannessi, Luca, Stienkemeier, Frank, Bruder, Lukas
Rok vydání:	2022
Předmět:	Physics - Atomic and Molecular Clusters
Druh dokumentu:	Working Paper
Popis:	Femtosecond extreme ultraviolet wave packet interferometry (XUV-WPI) was applied to study resonant inter-atomic Coulombic decay (ICD) in the HeNe dimer. The high demands on phase stability and sensitivity for vibronic XUV-WPI of molecular-beam targets are met using an XUV phase-cycling scheme. The detected quantum interferences exhibit vibronic dephasing and rephasing signatures along with an ultrafast decoherence assigned to the ICD process. A Fourier analysis reveals the molecular absorption spectrum with high resolution. The demonstrated experiment shows a promising route for the real-time analysis of ultrafast ICD processes with both high temporal and spectral resolution. Comment: 7 pages, 4 figures
Databáze:	arXiv
Externí odkaz:	http://arxiv.org/abs/2205.12885 Zobrazit plný text záznamu View this record from Arxiv