Structure Factor of a Phase Separating Binary Mixture with Natural and Forceful Interconversion of Species
Autor: | Longo, Thomas J., Shumovskyi, Nikolay A., Asadov, Salim M., Buldyrev, Sergey V., Anisimov, Mikhail A. |
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Rok vydání: | 2021 |
Předmět: | |
Druh dokumentu: | Working Paper |
Popis: | Using a modified Cahn-Hilliard-Cook theory for spinodal decomposition in a binary mixture that exhibits both diffusion and interconversion dynamics, we derive the time-dependent structure factor for concentration fluctuations. We compare the theory and obtain a qualitative agreement with simulations of the temporal evolution of the order parameter and structure factor in a nonequilibrium Ising/lattice-gas hybrid model in the presence of an external source of forceful interconversion. In particular, the characteristic size of the steady-state phase domain is predicted from the lower cut-off wavenumber of the amplification factor in the generalized spinodal-decomposition theory. Comment: Intended for J. Non Cryst. Solids: X |
Databáze: | arXiv |
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