The temperature-dependent chiral-induced spin selectivity effect: Experiments and theory

Autor:	Das, Tapan Kumar, Tassinari, Francesco, Naaman, Ron, Fransson, Jonas
Rok vydání:	2021
Předmět:	Condensed Matter - Mesoscale and Nanoscale Physics Condensed Matter - Other Condensed Matter Condensed Matter - Soft Condensed Matter
Zdroj:	J. Phys. Chem. C, 126, 3257 (2022)
Druh dokumentu:	Working Paper
DOI:	10.1021/acs.jpcc.1c10550
Popis:	The theoretical explanation for the chiral-induced spin selectivity effect, in which electrons' passage through a chiral system depends on their spin and the handedness of the system, remains vague. Although most experimental work was performed at room temperature, most of the proposed theories did not include vibrations. Here, we present temperature-dependent experiments and a theoretical model that captures all observations and provides spin polarization values that are consistent with the experimental results. The model includes vibrational contribution to the spin orbit coupling. It shows the importance of dissipation and the relation between the effect and the optical activity. Comment: 16 pages, 4 figure; submitted
Databáze:	arXiv
Externí odkaz:	http://arxiv.org/abs/2108.08037 Zobrazit plný text záznamu View this record from Arxiv