Coherent exciton-exciton interactions and exciton dynamics in a MoSe\textsubscript{2}/WSe\textsubscript{2} heterostructure

Autor: Purz, Torben L., Martin, Eric W., Rivera, Pasqual, Holtzmann, William G., Xu, Xiaodong, Cundiff, Steven T.
Rok vydání: 2021
Předmět:
Druh dokumentu: Working Paper
DOI: 10.1103/PhysRevB.104.L241302
Popis: Coherent coupling between excitons is at the heart of many-body interactions with transition metal dichalcogenide (TMD) heterostructures as an emergent platform for the investigation of these interactions. We employ multi-dimensional coherent spectroscopy on monolayer MoSe\textsubscript{2}/WSe\textsubscript{2} heterostructures and observe coherent coupling between excitons spatially localized in monolayer MoSe$_2$ and WSe$_2$. Through many-body spectroscopy, we further observe the absorption state arising from free interlayer electron-hole pairs. This observation yields a spectroscopic measurement of the interlayer exciton binding energy of about 250 meV.
Databáze: arXiv