Giant Rydberg excitons in Cu$_{2}$O probed by photoluminescence excitation spectroscopy

Autor: Versteegh, Marijn A. M., Steinhauer, Stephan, Bajo, Josip, Lettner, Thomas, Soro, Ariadna, Romanova, Alena, Gyger, Samuel, Schweickert, Lucas, Mysyrowicz, André, Zwiller, Val
Rok vydání: 2021
Předmět:
Druh dokumentu: Working Paper
DOI: 10.1103/PhysRevB.104.245206
Popis: Rydberg excitons are, with their ultrastrong mutual interactions, giant optical nonlinearities, and very high sensitivity to external fields, promising for applications in quantum sensing and nonlinear optics at the single-photon level. To design quantum applications it is necessary to know how Rydberg excitons and other excited states relax to lower-lying exciton states. Here, we present photoluminescence excitation spectroscopy as a method to probe transition probabilities from various excitonic states in cuprous oxide, and we show giant Rydberg excitons at $T=38$ mK with principal quantum numbers up to $n=30$, corresponding to a calculated diameter of 3 $\mu$m.
Comment: 11 pages, 4 figures
Databáze: arXiv