Field-tunable toroidal moment in a chiral-lattice magnet

Autor: Ding, Lei, Xu, Xianghan, Jeschke, Harald O., Bai, Xiaojian, Feng, Erxi, Alemayehu, Admasu Solomon, Kim, Jaewook, Huang, Feiting, Zhang, Qiang, Ding, Xiaxin, Harrison, Neil, Zapf, Vivien, Khomskii, Daniel, Mazin, Igor I., Cheong, Sang-Wook, Cao, Huibo
Rok vydání: 2021
Předmět:
Zdroj: Nature Communications 12, 5339 (2021)
Druh dokumentu: Working Paper
DOI: 10.1038/s41467-021-25657-6
Popis: A toroidal dipole moment appears independent of the electric and magnetic dipole moment in the multipole expansion of electrodynamics. It arises naturally from vortex-like arrangements of spins. Observing and controlling spontaneous long-range orders of toroidal moments are highly promising for spintronics but remain challenging. Here we demonstrate that a vortex-like spin configuration with a staggered arrangement of toroidal moments, a ferritoroidal state, is realized in a chiral triangular-lattice magnet BaCoSiO4. Upon applying a magnetic field, we observe multi-stair toroidal transitions correlating directly with metamagnetic transitions. We establish a first-principles microscopic Hamiltonian that explains both the formation of toroidal states and the metamagnetic toroidal transition as a combined effect of the magnetic frustration and the Dzyaloshinskii-Moriya interactions allowed by the crystallographic chirality in BaCoSiO4.
Databáze: arXiv