Magneto-optical determination of the carrier lifetime in coherent Ge(1-x)Sn(x)/Ge heterostructures

Autor: Vitiello, Elisa, Rossi, Simone, Broderick, Christopher A., Gravina, Giorgio, Balocchi, Andrea, Marie, Xavier, O'Reilly, Eoin P., Myronov, Maksym, Pezzoli, Fabio
Rok vydání: 2020
Předmět:
Zdroj: Phys. Rev. Applied 14, 064068 (2020)
Druh dokumentu: Working Paper
DOI: 10.1103/PhysRevApplied.14.064068
Popis: We present a magneto-optical study of the carrier dynamics in compressively strained Ge(1-x)Sn(x) films having Sn compositions up to 10% epitaxially grown on blanket Ge on Si (001) virtual substrates. We leverage the Hanle effect under steady-state excitation to study the spin-dependent optical transitions in presence of an external magnetic field. This allowed us to obtain direct access to the dynamics of the optically-induced carrier population. Our approach singled out that at cryogenic temperatures the effective lifetime of the photogenerated carriers in coherent Ge(1-x)Sn(x) occurs in the sub-ns time scale. Supported by a model estimate of the radiative lifetime, our measurements indicate that carrier recombination is dominated by non-radiative processes. Our results thus provide central information to advance the fundamental understanding of carrier kinetics in this novel direct-gap group-IV material system. Such knowledge can be a stepping stone in the quest for the implementation of Ge(1-x)Sn(x)-based functional devices.
Databáze: arXiv