| Autor: |
Benka, Georg, Bauer, Andreas, Schmakat, Philipp, Säubert, Steffen, Seifert, Marc, Jorba, Pau, Pfleiderer, Christian |
| Rok vydání: |
2020 |
| Předmět: |
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| Zdroj: |
Phys. Rev. Mater. 6, 044407(2022) |
| Druh dokumentu: |
Working Paper |
| DOI: |
10.1103/PhysRevMaterials.6.044407 |
| Popis: |
When suppressing the itinerant antiferromagnetism in chromium by doping with the isostructual itinerant ferromagnet iron, a dome of spin-glass behavior emerges around a putative quantum critical point at an iron concentration $x \approx 0.15$. Here, we report a comprehensive investigation of polycrystalline samples of Fe$_{x}$Cr$_{1-x}$ in the range $0.05 \leq x \leq 0.30$ using x-ray powder diffraction, magnetization, ac susceptibility, and neutron depolarization measurements, complemented by specific heat and electrical resistivity data for $x = 0.15$. Besides antiferromagnetic ($x < 0.15$) and ferromagnetic regimes ($0.15 \leq x$), we identify a dome of reentrant spin-glass behavior at low temperatures for $0.10 \leq x \leq 0.25$ that is preceded by a precursor phenomenon. Neutron depolarization indicates an increase of the size of ferromagnetic clusters with increasing $x$ and the Mydosh parameter $\phi$, inferred from the ac susceptibility, implies a crossover from cluster-glass to superparamagnetic behavior. Taken together, these findings consistently identify Fe$_{x}$Cr$_{1-x}$ as an itinerant-electron system that permits to study the evolution of spin-glass behavior of gradually varying character in unchanged crystalline environment. |
| Databáze: |
arXiv |
| Externí odkaz: |
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