Universal low-frequency vibrational modes in silica glasses

Autor: Bonfanti, Silvia, Guerra, Roberto, Mondal, Chandana, Procaccia, Itamar, Zapperi, Stefano
Rok vydání: 2020
Předmět:
Zdroj: Phys. Rev. Lett. 125, 085501 (2020)
Druh dokumentu: Working Paper
DOI: 10.1103/PhysRevLett.125.085501
Popis: It was recently shown that different simple models of glass formers with binary interactions define a universality class in terms of the density of states of their quasi-localized low-frequency modes. Explicitly, once the hybridization with standard Debye (extended) modes is avoided, a number of such models exhibit a universal density of state, depending on the mode frequencies as $D(\omega) \sim \omega^4$. It is unknown however how wide is this universality class, and whether it also pertains to more realistic models of glass formers. To address this issue we present analysis of the quasi-localized modes in silica, a network glass which has both binary and ternary interactions. We conclude that in 3-dimensions silica exhibits the very same frequency dependence at low frequencies, suggesting that this universal form is a generic consequence of amorphous glassiness.
Comment: 4 pages, 5 figures, Submitted in parallel to "Universality of the nonphononic vibrational spectrum across different classes of computer glasses" to arXiv on March 17th, 2020
Databáze: arXiv