Magnetic field effects on the quantum spin liquid behaviors of NaYbS$_2$

Autor: Wu, Jiangtao, Li, Jianshu, Zhang, Zheng, Liu, Changle, Gao, YongHao, Feng, Erxi, Deng, Guochu, Ren, Qingyong, Wang, Zhe, Chen, Rui, Embs, Jan, Zhu, Fengfeng, Huang, Qing, Xiang, Ziji, Chen, Lu, Wu, Yan, Choi, E. S., Qu, Zhe, Li, Lu, Wang, Junfeng, Zhou, Haidong, Su, Yixi, Wang, Xiaoqun, Chen, Gang, Zhang, Qingming, Ma, Jie
Rok vydání: 2020
Předmět:
Zdroj: Quantum Front 1, 13 (2022)
Druh dokumentu: Working Paper
DOI: 10.1007/s44214-022-00011-z
Popis: Spin-orbit coupling is an important ingredient to regulate the many-body physics, especially for many spin liquid candidate materials such as rare-earth magnets and Kitaev materials. The rare-earth chalcogenides NaYbCh$_2$ (Ch = O, S, Se) is a congenital frustrating system to exhibit the intrinsic landmark of spin liquid by eliminating both the site disorders between Na$^{+}$ and Yb$^{3+}$ ions with the big ionic size difference and the Dzyaloshinskii-Moriya interaction with the perfect triangular lattice of the Yb$^{3+}$ ions. The temperature versus magnetic-field phase diagram is established by the magnetization, specific heat, and neutron-scattering measurements. Notably, the neutron diffraction spectra and the magnetization curve might provide microscopic evidence for a series of spin configuration for in-plane fields, which include the disordered spin liquid state, 120$^{o}$ antiferromagnet, and one-half magnetization state. Furthermore, the ground state is suggested to be a gapless spin liquid from inelastic neutron scattering, and the magnetic field adjusts the spin orbit coupling. Therefore, the strong spin-orbit coupling in the frustrated quantum magnet substantially enriches low-energy spin physics. This rare-earth family could offer a good platform for exploring the quantum spin liquid ground state and quantum magnetic transitions.
Databáze: arXiv