Nonlinear quantum optics with trion-polaritons in 2D monolayers: conventional and unconventional photon blockade

Autor: Kyriienko, O., Krizhanovskii, D. N., Shelykh, I. A.
Rok vydání: 2019
Předmět:
Zdroj: Phys. Rev. Lett. 125, 197402 (2020)
Druh dokumentu: Working Paper
DOI: 10.1103/PhysRevLett.125.197402
Popis: We study a 2D system of trion-polaritons at the quantum level and demonstrate that for monolayer semiconductors they can exhibit a strongly nonlinear optical response. The effect is due to the composite nature of trion-based excitations resulting in their nontrivial quantum statistical properties, and enhanced phase space filling effects. We present the full quantum theory to describe the statistics of trion-polaritons, and demonstrate that the associated nonlinearity persists at the level of few quanta, where two qualitatively different regimes of photon antibunching are present for weak and strong single photon-trion coupling. We find that single photon emission from trion-polaritons becomes experimentally feasible in state-of-the-art transition metal dichalcogenide (TMD) setups. This can foster the development of quantum polaritonics using 2D monolayers as a material platform.
Comment: please see the related experiment in arXiv:1910.14636
Databáze: arXiv