Partial Antiferromagnetic Helical Order in Fe$_3$PO$_4$O$_3$

Autor: Sarkis, C. L., Tarne, M. J., Neilson, J. R., Cao, H. B., Coldren, E., Gelfand, M. P., Ross, K. A.
Rok vydání: 2019
Předmět:
Zdroj: Phys. Rev. B 101, 184417 (2020)
Druh dokumentu: Working Paper
DOI: 10.1103/PhysRevB.101.184417
Popis: Magnetic frustration in Fe$_3$PO$_4$O$_3$ has been shown to produce to an unusual magnetic state below T$_N = 163$ K, where incommensurate antiferromagnetic order is restricted to nanosized needle-like domains, as inferred from neutron powder diffraction. Here we show using single-crystal neutron diffraction that Fe$_3$PO$_4$O$_3$ does not exhibit a preferred ordering wavevector direction in the $ab$ plane despite having a well-defined ordering wavevector length. This results in the observation of continuous rings of scattering rather than satellite Bragg peaks. The lack of a preferred incommensurate ordering wavevector direction can be understood in terms of an antiferromagnetic Heisenberg model with nearest-neighbor ($J_1$) and second-neighbor ($J_2$) interactions, which produces a quasi-degenerate manifold of ordering wavevectors. This state appears to be similar to the partially ordered phase of MnSi, but in Fe$_3$PO$_4$O$_3$ arises in a frustrated antiferromagnet rather than a chiral ferromagnet.
Databáze: arXiv