Study of photoinduced valence dynamics in EuNi$_2$(Si$_{0.21}$Ge$_{0.79}$)$_2$ through time-resolved X-ray absorption spectroscopy

Autor: Yokoyama, Y., Kawakami, K., Hirata, Y., Takubo, K., Yamamoto, K., Abe, K., Mitsuda, A., Wada, H., Uozumi, T., Yamamoto, S., Matsuda, I., Mimura, K., Wadati, H.
Rok vydání: 2019
Předmět:
Zdroj: Phys. Rev. B 100, 115123 (2019)
Druh dokumentu: Working Paper
DOI: 10.1103/PhysRevB.100.115123
Popis: The photoinduced valence dynamics of EuNi$_2$(Si$_{0.21}$Ge$_{0.79}$)$_2$ are investigated using time-resolved X-ray absorption spectroscopy for Eu $M_5$-edge. Through the pump-probe technique with synchrotron X-ray and Ti:sapphire laser pulse, a photoinduced valence transition is observed from Eu$^{3+}$ to Eu$^{2+}$. Because the lifetime of a photoinduced state can be up to 3 ns, a metastable state is considered to be realized. By comparing the experimental results with the theoretical calculations, the photoinduced valence transition between Eu 4$f$ and conduction electrons is quantitatively evaluated.
Comment: 5 pages, 5 figures
Databáze: arXiv