Temperature-independent thermal radiation
Autor: | Shahsafi, Alireza, Roney, Patrick, Zhou, You, Zhang, Zhen, Xiao, Yuzhe, Wan, Chenghao, Wambold, Raymond, Salman, Jad, Yu, Zhaoning, Li, Jiarui, Sadowski, Jerzy T., Comin, Riccardo, Ramanathan, Shriram, Kats, Mikhail A. |
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Rok vydání: | 2019 |
Předmět: | |
Druh dokumentu: | Working Paper |
DOI: | 10.1073/pnas.1911244116 |
Popis: | Thermal emission is the process by which all objects at non-zero temperatures emit light, and is well-described by the classic Planck, Kirchhoff, and Stefan-Boltzmann laws. For most solids, the thermally emitted power increases monotonically with temperature in a one-to-one relationship that enables applications such as infrared imaging and non-contact thermometry. Here, we demonstrate ultrathin thermal emitters that violate this one-to-one relationship via the use of samarium nickel oxide (SmNiO3), a strongly correlated quantum material that undergoes a fully reversible, temperature-driven solid-state phase transition. The smooth and hysteresis-free nature of this unique insulator-to-metal (IMT) phase transition allows us to engineer the temperature dependence of emissivity to precisely cancel out the intrinsic blackbody profile described by the Stefan-Boltzmann law, for both heating and cooling. Our design results in temperature-independent thermally emitted power within the long-wave atmospheric transparency window (wavelengths of 8 - 14 um), across a broad temperature range of ~30 {\deg}C, centered around ~120 {\deg}C. The ability to decouple temperature and thermal emission opens a new gateway for controlling the visibility of objects to infrared cameras and, more broadly, new opportunities for quantum materials in controlling heat transfer. Comment: Main text and supplementary |
Databáze: | arXiv |
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