Local magnetism, magnetic order and spin freezing in the 'nonmetallic metal' FeCrAs

Autor: Huddart, B. M., Birch, M. T., Pratt, F. L., Blundell, S. J., Porter, D. G., Clark, S. J., Wu, W., Julian, S. R., Hatton, P. D., Lancaster, T.
Rok vydání: 2018
Předmět:
Zdroj: J. Phys.: Condens. Matter 31, 285803 (2019)
Druh dokumentu: Working Paper
DOI: 10.1088/1361-648X/ab151f
Popis: We present the results of x-ray scattering and muon-spin relaxation ($\mu^{+}$SR) measurements on the iron-pnictide compound FeCrAs. Polarized non-resonant magnetic x-ray scattering results reveal the 120$^\circ$ periodicity expected from the suggested three-fold symmetric, non-collinear antiferromagnetic structure. $\mu^+$SR measurements indicate a magnetically ordered phase throughout the bulk of the material below $T_\mathrm{N}$=105(5) K. There are signs of fluctuating magnetism in a narrow range of temperatures above $T_\mathrm{N}$ involving low-energy excitations, while at temperatures well below $T_\mathrm{N}$ behaviour characteristic of freezing of dynamics is observed, likely reflecting the effect of disorder in our polycrystalline sample. Using density functional theory we propose a distinct muon stopping site in this compound and assess the degree of distortion induced by the implanted muon.
Databáze: arXiv