Isospin-phonon coupling and Fano-interference in spin-orbit Mott insulator Sr2IrO4
Autor: | Samanta, Kousik, Rigitano, Danilo, Pagliuso, Pascoal Jose Giglio, Granado, Eduardo |
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Rok vydání: | 2018 |
Předmět: | |
Druh dokumentu: | Working Paper |
DOI: | 10.1063/1.5094912 |
Popis: | The isospin-phonon coupling in Sr2IrO4 is investigated by temperature dependent phonon Raman scattering. Anomalous behavior in the frequency of all studied optical phonons is observed below the magnetic transition temperature TN ~240 K. The strongest effect is detected for the A1g mode at 272 cm-1 associated with the modulation of the Ir-O-Ir bond angle. Additionally, the A1g mode at 560 cm-1 shows a Fano asymmetric lineshape sensitive to TN, supporting the existence of low-energy (~70 meV) electronic excitations that are renormalized by the magnetic order. These results reveal new aspects of the interaction between the crystal lattice and electronic degrees of freedom in this spin-orbit entangled Mott insulator. Comment: 5 pages and 6 figures |
Databáze: | arXiv |
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