Evidence for charge transfer and proximate magnetism in graphene/a-RuCl_3 heterostructures

Autor: Zhou, Boyi, Balgley, J., Lampen-Kelley, P., Yan, J. -Q., Mandrus, D. G., Henriksen, E. A.
Rok vydání: 2018
Předmět:
Zdroj: Physical Review B 100, 165426 (2019)
Druh dokumentu: Working Paper
DOI: 10.1103/PhysRevB.100.165426
Popis: We report a study of electronic transport in van der Waals heterostructures composed of flakes of the antiferromagnetic Mott insulator a-RuCl_3 placed on top of monolayer graphene Hall bars. While the zero-field transport shows a strong resemblance to that of isolated graphene, we find a consistently $p$-type Hall effect suggestive of multiband conduction, along with a non-monotonic and gate-voltage-dependent excursion of the resistivity at low temperatures that is reminiscent of transport in the presence of a magnetic phase transition. We interpret these data as evidence for charge transfer from graphene to a-RuCl_3 in an inhomogeneous device yielding both highly- and lightly-doped regions of graphene, while the latter shows a particular sensitivity to magnetism in the a-RuCl_3. Thus proximity to graphene is a means to access magnetic properties of thin layers of magnetic insulators.
Databáze: arXiv