Probing spin correlations using angle resolved photoemission in a coupled metallic/Mott insulator system

Autor: Sunko, V., Mazzola, F., Kitamura, S., Khim, S., Kushwaha, P., Clark, O. J., Watson, M., Markovic, I., Biswas, D., Pourovskii, L., Kim, T. K., Lee, T. -L., Thakur, P. K., Rosner, H., Georges, A., Moessner, R., Oka, T., Mackenzie, A. P., King, P. D. C.
Rok vydání: 2018
Předmět:
Zdroj: Sci.Adv. 6 (2020) eaaz0611
Druh dokumentu: Working Paper
DOI: 10.1126/sciadv.aaz0611
Popis: A nearly free electron metal and a Mott insulating state can be thought of as opposite ends of possibilities for the motion of electrons in a solid. In the magnetic oxide metal PdCrO$_{2}$, these two coexist as alternating layers. Using angle resolved photoemission, we surprisingly find sharp band-like features in the one-electron removal spectral function of the correlated subsystem. We show that these arise because a hole created in the Mott layer moves to and propagates in the metallic layer while retaining memory of the Mott layer's magnetism. This picture is quantitatively supported by a strong coupling analysis capturing the physics of PdCrO$_{2}$ in terms of a Kondo lattice Hamiltonian. Our findings open new routes to use the non-magnetic probe of photoemission to gain insights into the spin-susceptibility of correlated electron systems.
Databáze: arXiv