Microscopic Observation of Heavy Quasiparticle Formation in the Intermediate Valence Compound EuNi$_2$P$_2$: $^{31}$P NMR Study

Autor: Higa, Nonoka, Yogi, Mamoru, Kuroshima, Hiroko, Toji, Tatsuki, Niki, Haruo, Hiranaka, Yuichi, Nakamura, Ai, Nakama, Takao, Hedo, Masato, Ōnuki, Yoshichika
Rok vydání: 2018
Předmět:
Zdroj: J. Phys. Soc. Jpn. 87, 094708 (2018)
Druh dokumentu: Working Paper
DOI: 10.7566/JPSJ.87.094708
Popis: We report $^{31}$P NMR measurements under various magnetic fields up to 7 T for the intermediate valence compound EuNi$_2$P$_2$, which shows heavy electronic states at low temperatures. In the high-temperature region above 40 K, the Knight shift followed the Curie--Weiss law reflecting localized $4f$ states. In addition, the behavior corresponding to the temperature variation of the average valence of Eu was observed in the nuclear spin-lattice relaxation rate $1/T_1$. With the occurrence of the Kondo effect, $1/T_1$ was clearly reduced below 40 K, and the Knight shift becomes almost constant at low temperatures. From these results, the formation of heavy quasiparticles by the hybridization of Eu $4f$ electrons and conduction electrons was clarified from microscopic viewpoints. Furthermore, a characteristic spin fluctuation was observed at low temperatures, which would be associated with valence fluctuations caused by the intermediate valence state of EuNi$_2$P$_2$.
Comment: 7 pages, 5 figures
Databáze: arXiv