Spectroscopic signature of the $\mathbf{k}$-dependent electron-phonon coupling in $2H$-TaS$_2$

Autor: Wijayaratne, K., Zhao, J., Malliakas, C. D., Chung, D. Y., Kanatzidis, M. G., Chatterjee, U.
Rok vydání: 2018
Předmět:
Zdroj: Journal of Materials Chemistry C, V 5, pp 11310, 2017
Druh dokumentu: Working Paper
DOI: 10.1039/C7TC02641B
Popis: Our detailed Angle Resolved Photoemission Spectroscopy (ARPES) study of $2H$-TaS$_2$, a canonical incommensurate charge density wave (CDW) material, illustrates pronounced many-body renormalization in the system, which is manifested by the presence of multiple kink structures in the electronic dispersions. Temperature-dependent measurements reveal that these kink structures persist even at temperatures higher than the charge density wave transition temperature $\it{T}_{\text{cdw}}\,$ and the energy locations of the kinks are practically temperature-independent. Correlating kink energies with the published Raman scattering data and the theoretically calculated phonon spectrum of $2H$-TaS$_2$, we conclude phononic mechanism for these kinks. We have also detected momentum-anisotropy in the band renormalization, which in turn indicates momentum-dependence of the electron-phonon coupling of the system.
Comment: 6 pages, 3 figures
Databáze: arXiv