Quantum coherent control of the photo\-electron angular distribution in bichromatic ionization of atomic neon

Autor: Gryzlova, E. V., Grum-Grzhimailo, A. N., Staroselskaya, E. I., Douguet, N., Bartschat, K.
Rok vydání: 2017
Předmět:
Zdroj: Phys. Rev. A 97, 013420 (2018)
Druh dokumentu: Working Paper
DOI: 10.1103/PhysRevA.97.013420
Popis: We investigate the coherent control of the photo\-electron angular distribution in bichromatic atomic ionization. Neon is selected as target since it is one of the most popular systems in current gas-phase experiments with free-electron lasers (FELSs). In particular, we tackle practical questions, such as the role of the fine-structure splitting, the pulse length, and the intensity. Time-dependent and stationary perturbation theory are employed, and we also solve the time-dependent Schr\"odinger equation in a single-active electron model. We consider neon ionized by a FEL pulse whose fundamental frequency is in resonance with either $2p-3s$ or $2p-4s$ excitation. The contribution of the non\-resonant two-photon process and its potential constructive or destructive role for quantum coherent control is investigated.
Comment: 10 pages, 6 figures
Databáze: arXiv