Nonlinear photoionization of transparent solids: a nonperturbative theory obeying selection rules

Autor: Shcheblanov, N. S., Povarnitsyn, M. E., Terekhin, P. N., Guizard, S., Couairon, A.
Rok vydání: 2017
Předmět:
Zdroj: Phys. Rev. A 96, 063410 (2017)
Druh dokumentu: Working Paper
DOI: 10.1103/PhysRevA.96.063410
Popis: We provide a nonperturbative theory for photoionization of transparent solids. By applying a particular steepest-descent method, we derive analytical expressions for the photoionization rate within the two-band structure model, which consistently account for the $selection$ $rules$ related to the parity of the number of absorbed photons ($odd$ or $even$). We demonstrate the crucial role of the interference of the transition amplitudes (saddle-points), which in the semi-classical limit, can be interpreted in terms of interfering quantum trajectories. Keldysh's foundational work of laser physics [Sov. Phys. JETP 20, 1307 (1965)] disregarded this interference, resulting in the violation of $selection$ $rules$. We provide an improved Keldysh photoionization theory and show its excellent agreement with measurements for the frequency dependence of the two-photon absorption and nonlinear refractive index coefficients in dielectrics.
Databáze: arXiv