Tomonaga-Luttinger spin liquid in the spin-1/2 inequilateral diamond-chain compound K$_3$Cu$_3$AlO$_2$(SO$_4$)$_4$

Autor: Fujihala, M., Koorikawa, H., Mitsuda, S., Morita, K., Tohyama, T., Tomiyasu, K., Koda, A., Okabe, H., Itoh, S., Yokoo, T., Ibuka, S., Tadokoro, M., Itoh, M., Sagayama, H., Kumai, R., Murakami, Y., Nakamura, D.
Rok vydání: 2017
Předmět:
Zdroj: Scientific Reports 7 (2017) 16785
Druh dokumentu: Working Paper
DOI: 10.1038/s41598-017-16935-9
Popis: K$_3$Cu$_3$AlO$_2$(SO$_4$)$_4$ is a highly one-dimensional spin-1/2 inequilateral diamond-chain antiferromagnet. Spinon continuum and spin-singlet dimer excitations are observed in the inelastic neutron scattering spectra, which is in excellent agreement with a theoretical prediction: a dimer-monomer composite structure, where the dimer is caused by strong antiferromagnetic (AFM) coupling and the monomer forms an almost isolated quantum AFM chain controlling low-energy excitations. Moreover, muon spin rotation/relaxation spectroscopy shows no long-range ordering down to 90~mK, which is roughly three orders of magnitude lower than the exchange interaction of the quantum AFM chain. K$_3$Cu$_3$AlO$_2$(SO$_4$)$_4$ is, thus, regarded as a compound that exhibits a Tomonaga-Luttinger spin liquid behavior at low temperatures close to the ground state.
Databáze: arXiv