Beyond the effective mass approximation: predictive theory of the nonlinear optical response of conduction electrons

Autor: Yu, Shukai, Heffernan, Kate H., Talbayev, Diyar
Rok vydání: 2016
Předmět:
Zdroj: Phys. Rev. B 95, 125201 (2017)
Druh dokumentu: Working Paper
DOI: 10.1103/PhysRevB.95.125201
Popis: We present an experimental and computational study of the nonlinear optical response of conduction electrons to intense terahertz (THz) electric field. Our observations (saturable absorption and an amplitude-dependent group refractive index) can be understood on the qualitative level as the breakdown of the effective mass approximation. However, a predictive theoretical description of the nonlinearity has been missing. We propose a model based on the semiclassical electron dynamics, a realistic band structure, and the free electron Drude parameters to accurately calculate the experimental observables in InSb. Our results open a path to predictive modeling of the conduction-electron optical nonlinearity in semiconductors, metamaterials, as well as high-field effects in THz plasmonics.
Databáze: arXiv