Conductivity contrast and tunneling charge transport in the vortex-like ferroelectric domain patterns of multiferroic hexagonal YMnO3

Autor: Ruff, E., Krohns, S., Lilienblum, M., Meier, D., Fiebig, M., Lunkenheimer, P., Loidl, A.
Rok vydání: 2016
Předmět:
Zdroj: Phys. Rev. Lett. 118, 036803 (2017)
Druh dokumentu: Working Paper
DOI: 10.1103/PhysRevLett.118.036803
Popis: We deduce the intrinsic conductivity properties of the ferroelectric domain walls around the topologically protected domain vortex cores in multiferroic YMnO3. This is achieved by performing a careful equivalent-circuit analysis of dielectric spectra measured in single-crystalline samples with different vortex densities. The conductivity contrast between the bulk domains and the less conducting domain boundaries is revealed to reach up to a factor 500 at room temperature, depending on sample preparation. Tunneling of localized defect charge carriers is the dominant charge-transport process in the domain walls that are depleted of mo-bile charge carriers. This work demonstrates that via equivalent-circuit analysis, dielectric spectroscopy can provide valuable information on the intrinsic charge-transport properties of ferroelectric domain walls, which is of high relevance for the design of new domain-wall-based microelectronic devices.
Comment: 5 pages, 4 figures + 3 pages, 4 figures in Supplemental Material. Revised version as accepted for publication in Phys. Rev. Lett
Databáze: arXiv