Near-Infrared-Assisted Charge Control and Spin Readout of the Nitrogen-Vacancy Center in Diamond

Autor: Hopper, David A., Grote, Richard R., Exarhos, Annemarie L., Bassett, Lee C.
Rok vydání: 2016
Předmět:
Zdroj: Phys. Rev. B 94, 241201 (2016)
Druh dokumentu: Working Paper
DOI: 10.1103/PhysRevB.94.241201
Popis: We utilize nonlinear absorption to design all-optical protocols that improve both charge state initialization and spin readout for the nitrogen-vacancy (NV) center in diamond. Non-monotonic variations in the equilibrium charge state as a function of visible and near-infrared (NIR) optical power are attributed to competing multiphoton absorption processes. In certain regimes, multicolor illumination enhances the steady-state population of the NV's negative charge state above 90%. At higher NIR intensities, selective ionization of the singlet manifold facilitates a protocol for spin-to-charge conversion that dramatically enhances the spin readout fidelity. We demonstrate a 6-fold increase in the signal-to-noise ratio for single-shot spin measurements and predict an orders-of-magnitude experimental speedup over traditional methods for emerging applications in magnetometry and quantum information science using NV spins.
Comment: 5 pages, 4 figures, plus supplement
Databáze: arXiv