Onset of exciton-exciton annihilation in single layer black phosphorus
Autor: | Surrente, A., Mitioglu, A. A., Galkowski, K., Klopotowski, L., Tabis, W., Vignolle, B., Maude, D. K., Plochocka, P. |
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Rok vydání: | 2016 |
Předmět: | |
Zdroj: | Phys. Rev. B 94, 075425 (2016) |
Druh dokumentu: | Working Paper |
DOI: | 10.1103/PhysRevB.94.075425 |
Popis: | The exciton dynamics in monolayer black phosphorus is investigated over a very wide range of photoexcited exciton densities using time resolved photoluminescence. At low excitation densities, the exciton dynamics is successfully described in terms of a double exponential decay. With increasing exciton population, a fast, non-exponential component develops as exciton-exciton annihilation takes over as the dominant recombination mechanism under high excitation conditions. Our results identify an upper limit for the injection density, after which exciton-exciton annihilation reduces the quantum yield, which will significantly impact the performance of light emitting devices based on single layer black phosphorus. Comment: 6 pages, 5 figures |
Databáze: | arXiv |
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