First-order melting of a weak spin-orbit Mott insulator into a correlated metal
Autor: | Hogan, Tom, Yamani, Z., Walkup, D., Chen, Xiang, Dally, Rebecca, Ward, Thomas Z., Hill, John, Islam, Z., Madhavan, Vidya, Wilson, Stephen D. |
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Rok vydání: | 2015 |
Předmět: | |
Zdroj: | Physical Review Letters 114, 257203 (2015) |
Druh dokumentu: | Working Paper |
DOI: | 10.1103/PhysRevLett.114.257203 |
Popis: | The electronic phase diagram of the weak spin-orbit Mott insulator (Sr(1-x)Lax)3Ir2O7 is determined via an exhaustive experimental study. Upon doping electrons via La substitution, an immediate collapse in resistivity occurs along with a narrow regime of nanoscale phase separation comprised of antiferromagnetic, insulating regions and paramagnetic, metallic puddles persisting until x~0.04. Continued electron doping results in an abrupt, first-order phase boundary where the Neel state is suppressed and a homogenous, correlated, metallic state appears with an enhanced spin susceptibility and local moments. As the metallic state is stabilized, a weak structural distortion develops and suggests a competing instability with the parent spin-orbit Mott state. Comment: 5 pages, 4 figures |
Databáze: | arXiv |
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