Haydeeite: a spin-1/2 kagome ferromagnet

Autor: Boldrin, D., Fak, B., Enderle, M., Bieri, S., Ollivier, J., Rols, S., Manuel, P., Wills, A. S.
Rok vydání: 2015
Předmět:
Zdroj: Physical Review B 91 (2015) 220408(R)
Druh dokumentu: Working Paper
DOI: 10.1103/PhysRevB.91.220408
Popis: The mineral haydeeite, alpha-MgCu3(OD)6Cl2, is a S=1/2 kagome ferromagnet that displays long-range magnetic order below TC=4.2 K with a strongly reduced moment. Our inelastic neutron scattering data show clear spin-wave excitations that are well described by a Heisenberg Hamiltonian with ferromagnetic nearest-neighbor exchange J1=-38 K and antiferromagnetic exchange Jd=+11 K across the hexagons of the kagome lattice. These values place haydeeite very close to the quantum phase transition between ferromagnetic order and non-coplanar twelve-sublattice cuboc2 antiferromagnetic order. Diffuse dynamic short-range ferromagnetic correlations observed above TC persist well into the ferromagnetically ordered phase with a behavior distinct from critical scattering.
Databáze: arXiv