Itinerant ferromagnetism in the As 4$p$ conduction band of Ba$_{0.6}$K$_{0.4}$Mn$_{2}$As$_{2}$ identified by x-ray magnetic circular dichroism

Autor: Ueland, B. G., Pandey, Abhishek, Lee, Y., Sapkota, A., Choi, Y., Haskel, D., Rosenberg, R. A., Lang, J. C., Harmon, B. N., Johnston, D. C., Kreyssig, A., Goldman, A. I.
Rok vydání: 2015
Předmět:
Zdroj: Phys. Rev. Lett. 114, 217001 (2015)
Druh dokumentu: Working Paper
DOI: 10.1103/PhysRevLett.114.217001
Popis: X-ray magnetic circular dichroism (XMCD) measurements on single-crystal and powder samples of Ba$_{0.6}$K$_{0.4}$Mn$_{2}$As$_{2}$ show that the ferromagnetism below $T_{\textrm{C}}\approx$ 100 K arises in the As $4p$ conduction band. No XMCD signal is observed at the Mn x-ray absorption edges. Below $T_{\textrm{C}}$, however, a clear XMCD signal is found at the As $K$ edge which increases with decreasing temperature. The XMCD signal is absent in data taken with the beam directed parallel to the crystallographic $\textrm{c}$ axis indicating that the orbital magnetic moment lies in the basal plane of the tetragonal lattice. These results show that the previously reported itinerant ferromagnetism is associated with the As $4p$ conduction band and that distinct local-moment antiferromagnetism and itinerant ferromagnetism with perpendicular easy axes coexist in this compound at low temperature.
Comment: 6 pages; Supplemental Material Included; The text in version 2 is slightly different from the text in version 1
Databáze: arXiv