Suppression of 3D-ordering by defects in the $S=1/2$ frustrated chain magnet LiCuVO$_4$

Autor: Prozorova, L. A., Sosin, S. S., Svistov, L. E., Buettgen, N., Kemper, J. B., Reyes, A. P., Riggs, S., Petrenko, O. A., Prokofiev, A.
Rok vydání: 2015
Předmět:
Druh dokumentu: Working Paper
Popis: We report on a heat capacity study of high quality single crystal samples of \lcvo\ -- a frustrated spin $S=1/2$ chain system -- in magnetic field amounting to 3/4 of the saturation field. At low fields up to about 7~T, a linear temperature dependence of the specific heat, $C_p\propto T$, resulting from 1D magnetic correlations in the spin chains is followed upon cooling by a sharp lambda anomaly of the transition into a 3D helical phase with $C_p\propto T^3$ behavior at low temperature. The transition from a spin liquid into a spin-modulated (SM) phase at higher fields occurs via a hump-like anomaly which, as the temperature decreases further turns into a $C_p\propto T^2$ law distinctive for a quasi-2D system. We suggest an explanation for how nonmagnetic defects in the Cu$^{2+}$ chains can suppress 3D long-range ordering in the SM phase and leave it undisturbed in a helical phase.
Comment: 4 pages, 4 figures
Databáze: arXiv