Enhanced Harmonic Generation from M=1 aligned Ar+

Autor: Brown, A. C., van der Hart, Hugo W.
Rok vydání: 2013
Předmět:
Druh dokumentu: Working Paper
DOI: 10.1103/PhysRevA.88.033419
Popis: We investigate harmonic generation (HG) from ground-state Ar+ aligned with M=1 at a laser wavelength of 390-nm and intensity of 4x10(14) Wcm-2. Using time-dependent R-matrix theory, we find that an initial state with magnetic quantum number M=1 provides a 4-fold increase in harmonic yield over M=0. HG arises primarily from channels associated with the (3)Pe threshold of Ar2+, in contrast with M=0 for which channels associated with the excited, (1)De threshold dominate HG. Multichannel and multielectron interferences lead to a more marked suppression of HG for M=1 than M=0.
Comment: 5 pages, 3 figures. Accepted by Phys. Rev. A
Databáze: arXiv