Giant exchange bias and ferromagnetism in the CoO shell of Co/CoO-MgO core-shell nanoparticles

Autor: Ge, C. N., Wan, Xiangang, Pellegrin, E., Hu, Z., Zou, W. Q., Du, Y. W.
Rok vydání: 2012
Předmět:
Druh dokumentu: Working Paper
Popis: Using magnetron sputtering, we produced a series of Co/CoO-MgO nanoparticles on Si(100) substrates. High-resolution transmission electron microscopy (HRTEM) image shows that small isolated Co-clusters (core) covered with CoO (shells) with a size of a few nm embedded in a MgO matrix. Resistivity as a function of Co atomic ratio exhibits a distinct percolation threshold with a sharp decrease around 69% Co content. Across the threshold, the resistivity drops about 7 orders of magnitude. For a sample at this percolation critical threshold, we have observed a giant exchange bias field HE=2460 Oe at T= 2K, and using soft x-ray magnetic circular dichroism at the Co-L2,3 edge, we have detected a ferromagnetic (FM) signal originating from the antiferromagnetic CoO shell. Moreover, decreasing the Mg-impurities will reduce the FM signal from CoO shell (namely the uncompensated spin density) and the size of HE, thus directly support the uncompensated spin model.
Databáze: arXiv