First Passage Times for a Tracer Particle in Single File Diffusion and Fractional Brownian Motion

Autor: Sanders, Lloyd P., Ambjornsson, Tobias
Rok vydání: 2012
Předmět:
Zdroj: J. Chem. Phys. 136, 175103 (2012)
Druh dokumentu: Working Paper
DOI: 10.1063/1.4707349
Popis: We investigate the full functional form of the first passage time density (FPTD) of a tracer particle in a single-file diffusion (SFD) system whose population is: (i) homogeneous, i.e., all particles having the same diffusion constant and (ii) heterogeneous, with diffusion constants drawn from a heavy-tailed power-law distribution. In parallel, the full FPTD for fractional Brownian motion [fBm - defined by the Hurst parameter, 0= 1/3, as predicted by Molchan [1999] for fBm. When H<1/3, which includes homogeneous SFD (H=1/4), and heterogeneous SFD (H<1/4), the WFA fails to agree with any temporal scale of the simulations and Molchan's long-time result. SFD systems are compared to their fBm counter parts; and in the homogeneous system both scaled FPTDs agree on all temporal scales including also, the result by Molchan, thus affirming that SFD and fBm dynamics belong to the same universality class. In the heterogeneous case SFD and fBm results for heterogeneity-averaged FPTDs agree in the asymptotic time limit. The non-averaged heterogeneous SFD systems display a lack of self-averaging. An exponential with a power-law argument, multiplied by a power-law pre-factor is shown to describe well the FPTD for all times for homogeneous SFD and sub-diffusive fBm systems.
Comment: 29 pages, 5 figures
Databáze: arXiv
Externí odkaz: