Suppression of f-Electron Itinerancy in CeRu2Si2 by a Strong Magnetic Field

Autor: Matsuda, Y. H., Nakamura, T., Her, J. L., Michimura, S., Inami, T., Kindo, K., Ebihara, T.
Rok vydání: 2012
Předmět:
Druh dokumentu: Working Paper
DOI: 10.1103/PhysRevB.86.041109
Popis: The valence state of Ce in a canonical heavy fermion compound CeRu2Si2 has been investigated by synchrotron X-ray absorption spectroscopy at 1.8 K in high magnetic fields of up to 40 T. The valence was slightly larger than for the pure trivalent state (Ce3+: f1), as expected in heavy fermion compounds, and it decreased toward the trivalent state as the magnetic field was increased. The field-induced valence reduction indicates that the itinerant character of the 4f electrons in CeRu2Si2 was suppressed by a strong magnetic field. The suppression was gradual and showed characteristic magnetic field dependence, which reflects the metamagnetism around Hm \sim 8 T. The itinerant character persisted, even at 40 T (\sim 5Hm), suggesting that the Kondo bound state is continuously broken by magnetic fields and that it should completely collapse at fields exceeding 200 T.
Comment: 5 pages, 4 figures, accepted for publication as a Rapid Communication in Physical Review B
Databáze: arXiv