Stabilization of charge and orbital ordered states by antiferromagnetism in the A-site ordered YBaMn2O6
Autor: | Zhang, X. N., Choi, K. -Y., Lemmens, P., Nakajima, T., Ueda, Y. |
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Rok vydání: | 2009 |
Předmět: | |
Druh dokumentu: | Working Paper |
Popis: | We report on Raman scattering measurements of the A-site ordered YBaMn2O6 in the wide temperature range of 10-650K. Upon cooling almost all phonon modes show pronounced temperature dependencies of frequency, linewidth, and scattering intensity. This suggests that the octahedra tilting, Mn-O bond angles and lengths vary with temperature in a concerted way. The remarkable feature is that the high-temperature metallic and the charge and orbital ordered (CO-OO) states coexist down to T_N=195K. In the antiferromagnetic state zone-folded modes are induced by the CO-OO superstructure and the phonon modes undergo an anomalous softening and narrowing. Our results evidence that the CO-OO state is stabilized by the spin ordering for temperatures below T_N. Comment: 4 pages, 3 figures, added reference and corrections |
Databáze: | arXiv |
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