Suppression of the Superconducting Transition in RFeAsO1-xFx for R = Tb, Dy, Ho
Autor: | Rodgers, J. A., Penny, G. B. S., Marcinkova, A., Bos, J. W. G., Sokolov, D. A., Kusmartseva, A., Huxley, A. D., Attfield, J. P. |
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Rok vydání: | 2009 |
Předmět: | |
Zdroj: | Physical Review B80 052508 (2009) |
Druh dokumentu: | Working Paper |
Popis: | A suppression of superconductivity in the late rare earth RFeAsO1-xFx materials is reported. The maximum critical temperature (Tc) decreases from 51 K for R = Tb to 36 K for HoFeAsO0.9F0.1, which has been synthesised under 10 GPa pressure. This suppression is driven by a decrease in the Fe-As-Fe angle below an optimimum value of 110.6 degrees, as the angle decreases linearly with unit cell volume (V) across the RFeAsO1-xFx series. A crossover in electronic structure around this optimum geometry is evidenced by a change in sign of the compositional dTc/dV, from negative values for previously reported large R materials to positive for HoFeAsO0.9F0.1. Comment: accepted to PRB |
Databáze: | arXiv |
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