Coherent Stimulated X-ray Raman Spectroscopy; Attosecond Extension of RIXS
Autor: | Mukamel, Upendra Harbola Shaul |
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Rok vydání: | 2009 |
Předmět: | |
Druh dokumentu: | Working Paper |
Popis: | Spontaneous and stimulated resonant inelastic X-ray Raman scattering signals are calculated using the Keldysh-Schwinger closed-time path loop and expressed as overlaps of Doorway and Window electron-hole wavepackets. These are recast in terms of the one-particle Green's functions and expansion coefficients of configuration interaction singles for valence excitations, which can be obtained from standard electronic structure codes. Calculation for many-body states of ground and core-excited system is avoided. Comment: 10 pages and 4 figures. To be published in Physical Review B |
Databáze: | arXiv |
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