Anomalous circular polarization of magneto-photoluminescence from individual CdSe nanocrystals
Autor: | Htoon, H., Crooker, S. A., Furis, M., Jeong, S., Efros, Al. L., Klimov, V. I. |
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Rok vydání: | 2008 |
Předmět: | |
Zdroj: | Physical Review Letters 102, 017402 (2009) |
Druh dokumentu: | Working Paper |
DOI: | 10.1103/PhysRevLett.102.017402 |
Popis: | We study the low-temperature magneto-photoluminescence (PL) from individual CdSe nanocrystals. Nanocrystals having a small "bright" exciton fine structure splitting ($<$0.5 meV) exhibit a conventional left- and right-circularly polarized Zeeman PL doublet in applied magnetic fields. In contrast, nanocrystals with large fine structure splitting ($>$1 meV) show an anomalous magneto-PL polarization, wherein the lower-energy peak becomes circularly polarized with increasing field, while the higher-energy peak remains linearly polarized. This unusual behavior arises from strong mixing between the absorbing and emitting bright exciton levels due to strong anisotropic exchange interactions. Comment: 15 pages, 3 figures; submitted |
Databáze: | arXiv |
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