High-temperature magnetic insulating phase in ultrathin La0.67Sr0.33MnO3 films

Autor: Hans, Boschker, Jaap, Kautz, Evert P, Houwman, Wolter, Siemons, Dave H A, Blank, Mark, Huijben, Gertjan, Koster, Arturas, Vailionis, Guus, Rijnders
Rok vydání: 2011
Zdroj: Physical review letters. 109(15)
ISSN: 1079-7114
Popis: We present a study of the thickness dependence of magnetism and electrical conductivity in ultrathin La0.67Sr0.33MnO3 films grown on SrTiO3 (110) substrates. We found a critical thickness of 10 unit cells below which the conductivity of the films disappeared and simultaneously the Curie temperature increased, indicating a magnetic insulating phase at room temperature. These samples have a Curie temperature of about 560 K with a significant saturation magnetization of 1.2±0.2μ(B)/Mn. The canted antiferromagnetic insulating phase in ultra thin films of n10 coincides with the occurrence of a higher symmetry structural phase with a different oxygen octahedra rotation pattern. Such a strain engineered phase is an interesting candidate for an insulating tunneling barrier in room temperature spin polarized tunneling devices.
Databáze: OpenAIRE