Unusual diffusive effects on the ESR of Nd³⁺ ions in the tunable topologically nontrivial semimetal YBiPt

Autor: G G, Lesseux, T M, Garitezi, P F S, Rosa, C B R, Jesus, S B, Oseroff, J L, Sarrao, Z, Fisk, R R, Urbano, P G, Pagliuso, C, Rettori
Rok vydání: 2016
Zdroj: Journal of physics. Condensed matter : an Institute of Physics journal. 28(12)
ISSN: 1361-648X
Popis: Electron spin resonance (ESR) of diluted Nd(3+) ions in the topologically nontrivial semimetallic (TNSM) YBiPt compound is reported. The cubic YBiPt compound is a non-centrosymmetric half Heusler material which crystallizes in the F43m space group. The low temperature Nd(3+) ESR spectra showed a g-value of 2.66(4) corresponding to a Γ6 cubic crystal field Kramers' doublet ground state. Remarkably, the observed metallic and diffusive (Dysonian) Nd(3+) lineshape presented an unusual dependence with grain size, microwave power, Nd(3+) concentration and temperature. Moreover, the spin dynamic of the localized Nd(3+) ions in YBiPt was found to be characteristic of a phonon-bottleneck regime. It is claimed that, in this regime for YBiPt, phonons are responsible for mediating the diffusion of the microwave energy absorbed at resonance by the Nd(3+) ions to the thermal bath throughout the skin depth (δ ≃ μm). We argue that this is only possible because of the existence of highly mobile conduction electrons inside the skin depth of YBiPt that are strongly coupled to the phonons by spin-orbit coupling. Therefore, our unexpected ESR results point to a coexistence of metallic and insulating behaviors within the skin depth of YBiPt. This scenario is discussed in the light of the TNSM properties of this compound.
Databáze: OpenAIRE