Influence of anomalous changes in the crystal structure on the transport properties of YbNi1-xCuxAl series of alloys
| Autor: | Gandra, Flávio César Guimarães, 1954 |
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| Přispěvatelé: | UNIVERSIDADE ESTADUAL DE CAMPINAS |
| Rok vydání: | 2022 |
| Předmět: | |
| Zdroj: | Repositório da Produção Científica e Intelectual da Unicamp Universidade Estadual de Campinas (UNICAMP) instacron:UNICAMP |
| Popis: | Results of the transport properties of the YbNi1-xCuxAl (x = 0, 0.2, 0.5, 0.8 and 1.0) series of alloys are reported. The previous analysis of X-ray diffraction patterns indicates that all compounds crystallize in the hexagonal ZrNiAl structure with a linear behavior of the unit cell volume as a function of the Cu concentration (x). This is not found in the unit cell parameters, showing a discontinuity between x = 0.5 and 0.8. Such discontinuities affect the behavior of the electrical resistivity, in which the position of the minimum temperature changes from 95 K to 175 K, and a rise in the low temperature slope in the magnetic contribution (with -lnT dependence) from 21 mu omega cm to 212 mu omega cm is observed. In addition, the electronic coefficient of the specific heat increases almost twofold from 125 mJ/mol center dot K-2 (x = 0.5) to 246 mJ/mol center dot K-2 (x = 0.8). These changes are attributed to the variation of the distance between Yb and transition metals (Ni and Cu) along the series and the different electronic properties of the transition metals (Ni and Cu) FUNDAÇÃO DE AMPARO À PESQUISA DO ESTADO DE SÃO PAULO - FAPESP Aberto |
| Databáze: | OpenAIRE |
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