Green ammonia synthesis using CeO2/RuO2 nanolayers on vertical graphene catalyst via electrochemical route in alkaline electrolyte

Autor: Ju, H, Seo, DH, Chung, S, Mao, X, An, B-S, Musameh, M, Gengenbach, TR, Shon, H, Du, A, Bendavid, A, Ostrikov, KK, Yoon, HC, Lee, J, Giddey, S
Jazyk: angličtina
Rok vydání: 2022
Předmět:
Popis: The electrochemical synthesis of ammonia at ambient temperature and pressure has the potential to replace the conventional process for the production of ammonia. However, the low ammonia yield and poor long-term stability of catalysts for the synthesis of ammonia hinders the application of this technology. Herein, we endeavored to tackle this challenge by synthesizing 3-D vertical graphene (VG) on Ni foam via a one-step, low-temperature plasma process, which offered high conductivity and large surface area. Subsequently, the vertical graphene on Ni foam was loaded with nanolayers of ruthenium oxide (RuO2, ∼2 nm) and cerium oxide (CeO2
Databáze: OpenAIRE