The VATO project An original methodology to study the transfer of tritium as HT and HTO in grassland ecosystem
| Autor: | Mehdi Morillon, D. Maro, S. Le Dizès, O. Connan, C. Aulagnier, Luc Solier, C. Cossonnet, O. Cazimajou, C Voiseux, M. Rozet, Bruno Fiévet, P. Laguionie, D. Hébert, M. Lamotte, C. Godinot, F. Vermorel |
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| Přispěvatelé: | PRP-ENV/SERIS/LRTE, Laboratoire de Recherche sur les Transferts des radionucléides dans l'Environnement, Institut de Radioprotection et de Sûreté Nucléaire (IRSN), PSE-ENV/SRTE/LRC, PRP-ENV/STEME/LMRE, Laboratoire de Mesure de la Radioactivité dans l’Environnement |
| Jazyk: | angličtina |
| Rok vydání: | 2017 |
| Předmět: |
010504 meteorology & atmospheric sciences
Health Toxicology and Mutagenesis [SDV]Life Sciences [q-bio] 010501 environmental sciences Tritium 7. Clean energy 01 natural sciences Rainwater harvesting Nuclear industry Radiation Monitoring Environmental Chemistry Waste Management and Disposal 0105 earth and related environmental sciences Nuclear fuel business.industry Ecology Environmental engineering General Medicine Nuclear power Pollution Grassland Nuclear facilities Nuclear reprocessing Models Chemical 13. Climate action Air Pollutants Radioactive Environmental science business Grassland ecosystem |
| Zdroj: | Journal of Environmental Radioactivity Journal of Environmental Radioactivity, Elsevier, 2017, 167, pp.235-248. ⟨10.1016/j.jenvrad.2016.10.016⟩ |
| ISSN: | 0265-931X 1879-1700 |
| Popis: | International audience; Tritium (3H) is mainly released into the environment by nuclear power plants, military nuclear facilities and nuclear reprocessing plants. The construction of new nuclear facilities in the world as well as the evolution of nuclear fuel management might lead to an increase of 3H discharges from the nuclear industry. The VATO project was set up by IRSN (Institut de Radioprotection et de Sûreté Nucléaire) and EDF (Electricité de France) to reduce the uncertainties in the knowledge about transfers of 3H from an atmospheric source (currently releasing HT and HTO) to a grassland ecosystem. A fully instrumented technical platform with specifically designed materials was set up downwind of the AREVA NC La Hague reprocessing plant (Northwest of the France). This study, started in 2013, was conducted in four main steps to provide an hourly data set of 3H concentrations in the environment, adequate to develop and/or validate transfer models. It consisted first in characterizing the physico-chemical forms of 3H present in the air around the plant. Then, 3H transfer kinetics to grass were quantified regarding contributions from various compartments of the environment. For this purpose, an original experimental procedure was provided to take account for biases due to rehydration of freeze-dried samples for the determination of OBT activity concentrations in biological samples. In a third step, the 3H concentrations measured in the air and in rainwater were reconstructed at hourly intervals. Finally, a data processing technique was used to determine the biological half-lives of OBT in grass. © 2016 Elsevier Ltd |
| Databáze: | OpenAIRE |
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