Exceeding Single-Pass Equilibrium with Integrated Absorption Separation for Ammonia Synthesis Using Renewable Energy—Redefining the Haber-Bosch Loop

Autor: Smith, C, Torrente-Murciano, L
Přispěvatelé: Torrente-Murciano, L [0000-0002-7938-2587], Apollo - University of Cambridge Repository
Rok vydání: 2021
Předmět:
DOI: 10.17863/cam.73869
Popis: The synthesis of ammonia through the Haber-Bosch process has been at the foundation of the chemical industry for over 100 years, but when the energy and feedstock sources switch from fossil fuels to renewable electricity, the process needs to be reimagined. Herein, the successful integration of ammonia synthesis and separation is demonstrated in a recycle-less process setting the foundations of green ammonia technology. The ruthenium-based catalyst uses a nanostructured CeO2 support and Cs electronic promotion to remove hydrogen and ammonia inhibition, respectively, creating a catalyst with low-temperature (
Databáze: OpenAIRE