Tunable spin-valley coupling in layered polar Dirac metals

Autor: Hideaki Sakai, H. Murakawa, Masashi Tokunaga, Masakazu Matsubara, Atsushi Miyake, Kazuhiko Kuroki, Masaki Kondo, Tatsuhiro Kojima, Ryosuke Kurihara, Daiki Sekine, Masayuki Ochi, Noriaki Hanasaki
Jazyk: angličtina
Rok vydání: 2021
Předmět:
Zdroj: Communications Materials, Vol 2, Iss 1, Pp 1-7 (2021)
ISSN: 2662-4443
Popis: In non-centrosymmetric metals, spin-orbit coupling (SOC) induces momentum-dependent spin polarization at the Fermi surfaces. This is exemplified by the valley-contrasting spin polarization in monolayer transition metal dichalcogenides (TMDCs) with in-plane inversion asymmetry. However, the valley configuration of massive Dirac fermions in TMDCs is fixed by the graphene-like structure, which limits the variety of spin-valley coupling. Here, we show that the layered polar metal BaMn$X_2$ ($X =$Bi, Sb) hosts tunable spin-valley-coupled Dirac fermions, which originate from the distorted $X$ square net with in-plane lattice polarization. We found that in spite of the larger SOC, BaMnBi$_2$ has approximately one-tenth the lattice distortion of BaMnSb$_2$, from which a different configuration of spin-polarized Dirac valleys is theoretically predicted. This was experimentally observed as a clear difference in the Shubnikov-de Haas oscillation at high fields between the two materials. The chemically tunable spin-valley coupling in BaMn$X_2$ makes it a promising material for various spin-valleytronic devices.
Comment: 25 pages, 4 figures. Published in Communications Materials
Databáze: OpenAIRE