Trace element and isotope deposition across the air–sea interface: progress and research needs
Autor: | William M. Landing, Christopher T. Hayes, Peter L. Morton, M.M.P. van Hulten, Marie Cheize, N. Rogan, Susanne Fietz, Géraldine Sarthou, R. Shelley, Alan M. Shiller, Eva Bucciarelli, Z. Shi, David Kadko, Alex R. Baker |
---|---|
Přispěvatelé: | Centre for Ocean and Atmospheric Sciences [Norwich] (COAS), School of Environmental Sciences [Norwich], University of East Anglia [Norwich] (UEA)-University of East Anglia [Norwich] (UEA), Department of Earth, Ocean and Atmospheric Science [Tallahassee] (FSU | EOAS), Florida State University [Tallahassee] (FSU), Laboratoire des Sciences de l'Environnement Marin (LEMAR) (LEMAR), Institut de Recherche pour le Développement (IRD)-Institut Français de Recherche pour l'Exploitation de la Mer (IFREMER)-Université de Brest (UBO)-Institut Universitaire Européen de la Mer (IUEM), Institut de Recherche pour le Développement (IRD)-Institut national des sciences de l'Univers (INSU - CNRS)-Université de Brest (UBO)-Centre National de la Recherche Scientifique (CNRS)-Institut national des sciences de l'Univers (INSU - CNRS)-Université de Brest (UBO)-Centre National de la Recherche Scientifique (CNRS)-Centre National de la Recherche Scientifique (CNRS), Université de Brest (UBO), Department of Earth Sciences [Stellenbosch], Stellenbosch University, University of Southern Mississippi (USM), Florida International University [Miami] (FIU), Helmholtz Centre for Ocean Research [Kiel] (GEOMAR), School of Geography, Earth and Environmental Sciences [Birmingham], University of Birmingham [Birmingham], Laboratoire des Sciences du Climat et de l'Environnement [Gif-sur-Yvette] (LSCE), Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ), Institut de Recherche pour le Développement (IRD)-Institut national des sciences de l'Univers (INSU - CNRS)-Université de Brest (UBO)-Centre National de la Recherche Scientifique (CNRS)-Institut de Recherche pour le Développement (IRD)-Institut national des sciences de l'Univers (INSU - CNRS)-Université de Brest (UBO)-Centre National de la Recherche Scientifique (CNRS)-Centre National de la Recherche Scientifique (CNRS), Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS) |
Jazyk: | angličtina |
Rok vydání: | 2016 |
Předmět: |
anthropogenic aerosols
atmospheric chemistry 010504 meteorology & atmospheric sciences biogeochemical impacts General Mathematics Geotraces chibido General Physics and Astronomy Flux sediment resuspension Review Article 010501 environmental sciences Mineral dust Atmospheric sciences air–sea exchange 01 natural sciences soluble organic-matter north-atlantic ocean dust deposition iron solubility 14. Life underwater Solubility 0105 earth and related environmental sciences mineral dust [SDU.OCEAN]Sciences of the Universe [physics]/Ocean Atmosphere dissolved aluminum trace element solubility ACL atmospheric deposition General Engineering Trace element air-sea exchange Articles Aerosol Deposition (aerosol physics) Oceanography 13. Climate action Atmospheric chemistry metal concentrations west atlantic [SDE.BE]Environmental Sciences/Biodiversity and Ecology |
Zdroj: | Philosophical Transactions of the Royal Society A: Mathematical, Physical and Engineering Sciences Philosophical Transactions of the Royal Society A: Mathematical, Physical and Engineering Sciences, Royal Society, The, 2016, 374 (2081), pp.20160190. ⟨10.1098/rsta.2016.0190⟩ Philosophical transactions. Series A, Mathematical, physical, and engineering sciences Philosophical Transactions Of The Royal Society A-mathematical Physical And Engineering Sciences (1364-503X) (Royal Soc), 2016-11, Vol. 374, N. 2081, P. 1-17 Philosophical Transactions of the Royal Society A: Mathematical, Physical and Engineering Sciences, 374 (2081). p. 20160190. Philosophical Transactions of the Royal Society A: Mathematical, Physical and Engineering Sciences, 2016, 374 (2081), pp.20160190. ⟨10.1098/rsta.2016.0190⟩ |
ISSN: | 1364-503X 1471-2962 |
Popis: | WOS:000391139900018; International audience; The importance of the atmospheric deposition of biologically essential trace elements, especially iron, is widely recognized, as are the difficulties of accurately quantifying the rates of trace element wet and dry deposition and their fractional solubility. This paper summarizes some of the recent progress in this field, particularly that driven by the GEOTRACES, and other, international research programmes. The utility and limitations of models used to estimate atmospheric deposition flux, for example, from the surface ocean distribution of tracers such as dissolved aluminium, are discussed and a relatively new technique for quantifying atmospheric deposition using the short-lived radionuclide beryllium-7 is highlighted. It is proposed that this field will advance more rapidly by using a multi-tracer approach, and that aerosol deposition models should be ground-truthed against observed aerosol concentration data. It is also important to improve our understanding of the mechanisms and rates that control the fractional solubility of these tracers. Aerosol provenance and chemistry (humidity, acidity and organic ligand characteristics) play important roles in governing tracer solubility. Many of these factors are likely to be influenced by changes in atmospheric composition in the future. Intercalibration exercises for aerosol chemistry and fractional solubility are an essential component of the GEOTRACES programme. This article is part of the themed issue 'Biological and climatic impacts of ocean trace element chemistry'. |
Databáze: | OpenAIRE |
Externí odkaz: |